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Shcherbakov, Maxim R.; Zhang, Haizhong; Tripepi, Michael; Sartorello, Giovanni; Talisa, Noah; AlShafey, Abdallah; Fan, Zhiyuan; Twardowski, Justin; Krivitsky, Leonid A.; Kuznetsov, Arseniy I.; et al (, Nature Communications)Abstract High harmonic generation (HHG) opens a window on the fundamental science of strong-field light-mater interaction and serves as a key building block for attosecond optics and metrology. Resonantly enhanced HHG from hot spots in nanostructures is an attractive route to overcoming the well-known limitations of gases and bulk solids. Here, we demonstrate a nanoscale platform for highly efficient HHG driven by intense mid-infrared laser pulses: an ultra-thin resonant gallium phosphide (GaP) metasurface. The wide bandgap and the lack of inversion symmetry of the GaP crystal enable the generation of even and odd harmonics covering a wide range of photon energies between 1.3 and 3 eV with minimal reabsorption. The resonantly enhanced conversion efficiency facilitates single-shot measurements that avoid material damage and pave the way to study the controllable transition between perturbative and non-perturbative regimes of light-matter interactions at the nanoscale.more » « less
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Shcherbakov, Maxim R.; Sartorello, Giovanni; Tripepi, Michael; AlShafey, Abdullah; Bosch, Melissa; Talisa, Noah; Chowdhury, Enam; Shvets, Gennady (, Conference on Lasers and Electro-Optics: Science and Innovations)
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Mueller, Sara M; Kim, Dongjoon; McMillan, Stephen R; Tjung, Steven J; Repicky, Jacob J; Gant, Stephen; Lang, Evan; Bergmann, Fedor; Werner, Kevin; Chowdhury, Enam; et al (, Journal of Physics: Condensed Matter)null (Ed.)
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